Overnight tomato shriveling

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Location
Missouri
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Hello!

We have been faithfully caring for our tomato plants since we started them from seed (with a grow light) several months ago, but all of a sudden have hit some trouble.

We had been dealing with aphids, and had been just removing them by hand. I’ve included a couple pictures of how the tomatoes looked a week ago.

We wanted a more efficient solution, so we recently sprayed them with Neem oil (pictured below). We sprayed in the evening, and also pruned the lower branches at the same time.

The next morning, the plants looked noticeably worse with curling leaves, and we watered them. They have gotten worse, and I’ve included several pictures of how they look now.

Could the Neem have caused this? What would be the best thing to do here?

Thank you for your time and your help!
 

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